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Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 53-62 doi: 10.1007/s11783-014-0728-z

摘要： Understanding the trends in PM levels is essential for formulating clean air plans. This paper analyzes PM data from various published sources for the years 2000 to 2010 in the Pearl River Delta Economic Zone (PRDEZ). The long-term variation in PM mass concentration is analyzed. Results show that PM , organic carbon (OC), elemental carbon (EC), and show a similar trend, increasing before 2005 and then decreasing slightly. The annual average PM concentration ranges from 49.1 μg·m in 2000 to 64.3 μg·m in 2010, with a peak of 84.1 μg·m in 2004. None of these 11 years meets the new National Ambient Air Quality standard (NAAQS) for PM (35 μg·m ). Overall average concentrations of OC, EC, and are 13.0, 6.5, and 11.8 μg·m , respectively. and respectively have concentrations of 1.5 μg·m and 2.9 μg·m in 2000 and 6.4 μg·m and 5.3 μg·m in 2010, with a statistically significant average annual trend of+ 0.2 μg·m ·yr and+ 0.1 μg·m ·yr . In certain geographic regions, OC and EC contribute most of the PM , while in other regions secondary water-soluble ions are more important. In general, OC and are the dominant components of PM , contributing 20.6% and 18.6%, respectively. These results provide, for the first time, a better understanding of the long-term PM characteristics and trends, on a species-by-species basis, in the PRDEZ. The results indicate that PM abatement needs to prioritize secondary species.

关键词： long-term trends     fine particulate matter     chemical components     Pearl River Delta Economic Zone (PRDEZ)    

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Online single particle analysis of chemical composition and mixing state of crop straw burning particles

Juntao HUO,Xiaohui LU,Xinning WANG,Hong CHEN,Xingnan YE,Song Gao,Deborah S. Gross,Jianmin CHEN,Xin YANG

《环境科学与工程前沿（英文）》 2016年 第10卷 第2期   页码 244-252 doi: 10.1007/s11783-015-0768-z

摘要： Fresh straw burning (SB) particles were generated in the laboratory by the combustion of rice straw and corn straw. The chemical composition and mixing state of the fresh SB particles were investigated by an Aerosol Time-of-Flight Mass Spectrometer (ATOFMS). Based on the mass spectral patterns, the SB particles were clustered into four major types: Salt, Organic Carbon (OC), Elemental Carbon (EC), and internally mixed particles of EC and OC (EC-OC). In addition, particles containing ash, polycyclic aromatic hydrocarbons, heavy metals or nicotine were also observed. Physical and chemical changes of the SB particles immediately after the emission were analyzed with highly time-resolved data. During the aging processes, the average particle size increased steadily. Freshly emitted organic compounds were gradually oxidized to more oxygenated compounds in the OC-containing particles. Meanwhile, an important displacement reaction (2KCl+ → K SO + 2Cl ) was observed. The marker ions for SB particles were optimized and applied to identify the SB particles in the ambient atmosphere. The fluctuation of the number fraction of ambient SB particles sorted by ATOFMS agrees well with that of water soluble K measured by an online ion chromatography, demonstrating that the optimized marker ions could be good tracers for SB particles in field measurements.

关键词： crop straw burning particles     mixing state     aging process     ATOFMS     ion markers    

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Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganese

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

《能源前沿（英文）》 2017年 第11卷 第3期   页码 365-373 doi: 10.1007/s11708-017-0500-8

摘要： Lithium manganese oxide (LiMn O ) is a principal cathode material for high power and high energy density electrochemical storage on account of its low cost, non-toxicity, and ease of preparation relative to other cathode materials. However, there are well-documented problems with capacity fade of lithium ion batteries containing LiMn O . Experimental observations indicate that the manganese content of the electrolyte increases as an electrochemical cell containing LiMn O ages, suggesting that active material loss by dissolution of divalent manganese from the LiMn O surface is the primary reason for reduced cell life in LiMn O batteries. To improve the retention of manganese in the active material, it is key to understand the reactions that occur at the cathode surface. Although a thin layer of electrolyte decomposition products is known to form at the cathode surface, the speciation and reaction mechanisms of Mn in this interface layer are not yet well understood. To bridge this knowledge gap, reactive force field (ReaxFF) based molecular dynamics was applied to investigate the reactions occurring at the LiMn O cathode surface and the mechanisms that lead to manganese dissolution. The ReaxFFMD simulations reveal that the cathode-electrolyte interface layer is composed of oxidation products of electrolyte solvent molecules including aldehydes, esters, alcohols, polycarbonates, and organic radicals. The oxidation reaction pathways for the electrolyte solvent molecules involve the formation of surface hydroxyl species that react with exposed manganese atoms on the cathode surface. The presence of hydrogen fluoride (HF) induces formation of inorganic metal fluorides and surface hydroxyl species. Reaction products predicted by ReaxFF-based MD are in agreement with experimentally identified cathode-electrolyte interface compounds. An overall cathode-electrolyte interface reaction scheme is proposed based on the molecular simulation results.

关键词： lithium manganese oxide batteries     reactive force field (ReaxFF)     cathode-electrolyte interface layer     molecular dynamics    

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Preliminary study of trace element emissions and control during coal combustion

ZHANG Junying, ZHAO Yongchun, DING Feng, ZENG Hancai, ZHENG Chuguang

《能源前沿（英文）》 2007年 第1卷 第3期   页码 273-279 doi: 10.1007/s11708-007-0038-2

摘要： Hazardous trace element emissions have caused serious harm to human health in China. Several typical high-toxic trace element coals were collected from different districts and were used to investigate the emission characteristics of toxic trace elements (As, Se, Cr, Hg) and to explore preliminary control methods. Coal combustion tests were conducted in several bench-scale furnaces including drop tube furnace (DTF), circulating fluidized bed (CFB) combustion furnace, and fixed-bed combustion furnace. Calcium oxide was used to control the emission of arsenic and selenium. The granular activated carbons (AC) and activated-carbon fibers (ACF) were used to remove mercury in the flue gas from coal combustion. The chemical composition and trace element contents of ash and particulate matter (PM) were determined by X-ray fluorescence (XRF) spectrometry and inductively coupled plasma-atomic emission spectrometry (ICP-AES), respectively. The speciation and concentration of mercury were investigated using the Ontario-Hydro method. X-ray diffraction spectrometry (XRD) was used to determine the mineral composition of production during combustion experiments. With the addition of a calcium-based sorbent, arsenic concentration in PM sharply decreased from 0.25–0.11 mg/m. In fixed-bed combustion of coal, the retention rates of selenium volatiles were between 11.6% and 50.7% using lime. In the circulating fluidized-bed combustion of coal, the content of selenium in ash from the chimney was reduced to one-fourth of its original value and that in leaching water from the chimney decreased by two orders of magnitude using lime. Calcium-based sorbent is an effective additive to control the emission of As and Se during coal combustion. The emission of chromium is influenced by the occurrence mode of Cr in coal. Chromium emission in PM during coal combustion is 55.5 and 34.7 μg/m for Shenbei coal and mixed Pingdingshan coal, respectively. The adsorptive capacity of granular activated carbon for Hg is significantly enhanced through ZnCl-impregnation. The activated carbon fibers showed decent efficiency in mercury adsorption, on which surface oxygen complex showed positive effects on mercury adsorption.

关键词： Pingdingshan     occurrence     plasma-atomic emission     chemical composition     Several typical    

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“Composition” and regularisation of architectural production in contemporary China

Hua LI

《结构与土木工程前沿（英文）》 2010年 第4卷 第4期   页码 465-473 doi: 10.1007/s11709-010-0097-z

摘要： The purpose of this paper is to explore how the “Beaux-Arts” “composition” sustained the constitution of design principles for architectural production in China in the last two decades of the twentieth century. “Composition”, a key technique of the “Beaux-Arts” system, is not a simple act of “putting elements together” into a unified whole, but also relates to an array of different “constructions” of architectural knowledge which regulate and sustain the act of design. Through analysing the structure of three “textbooks” published in the early 1980s, this paper examines three aspects of the “constructions”: the setting up of the principles for governing architectural forms, regularisation of design methods and approaches for architectural practice, and the construction of a “tradition” for the expression of “Chineseness”.

关键词： composition     “Beaux-Arts”     regulate     architectural production    

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Calorie restriction and its impact on gut microbial composition and global metabolism

Xiaojiao Zheng, Shouli Wang, Wei Jia

《医学前沿（英文）》 2018年 第12卷 第6期   页码 634-644 doi: 10.1007/s11684-018-0670-8

摘要：

Calorie restriction (CR) is a dietary regimen that reduces calorie intake without incurring malnutrition or a reduction in essential nutrients. It has long been recognized as a natural strategy for promoting health, extending longevity, and prevents the development of metabolic and age-related diseases. In the present review, we focus on the general effect of CR on gut microbiota composition and global metabolism. We also propose mechanisms for its beneficial effect. Results showed that probiotic and butyrate-producing microbes increased their relative abundance, whereas proinflammatory strains exhibited suppressed relative abundance following CR. Analyses of the gut microbial and host metabolisms revealed that most host microbial co-metabolites were changed due to CR. Examples of dramatic CR-induced changes in host metabolism included a decrease in the rate of lipid biosynthesis and an increase in the rates of fatty acid catabolism, β-oxidation, glycogenolysis, and gluconeogenesis. The observed phenotypes and the further verification of the direct link between gut microbiota and metabolome may benefit patients that are at risk for developing metabolic disease. Thus, improved gut microbiota composition and metabolome are potential biomarkers for determining the effectiveness of dietary interventions for age-related and metabolic diseases.

关键词： caloric restriction     gut microbiota     metabolome    

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Sensitivity analysis of a methanol and power polygeneration system fueled with coke oven gas and coal gas

Guoqiang ZHANG, Lin GAO, Hongguang JIN, Rumou LIN, Sheng LI

《化学科学与工程前沿（英文）》 2010年 第4卷 第4期   页码 491-497 doi: 10.1007/s11705-010-0511-z

摘要： The sensitivity analysis of a polygeneration energy system fueled with duo fuel of coke oven gas and coal gas is performed in the study, and the focus is put on the relations among syngas composition, conversation rate and performance. The impacts of the system configuration together with the fuel composition on the performance are investigated and discussed from the point of cascading utilization of fuel chemical energy. First, the main parameters affecting the performance are derived along with the analysis of the system configuration and the syngas composition. After the performance is being simulated by means of the Aspen Plus process simulator of version 11.1, the variation of the performance due to the composition of syngas and the conversion rate of chemical subsystem is obtained and discussed. It is obtained from the result that the proper conversion rate of the chemical subsystem according to the specific syngas composition results in better performance. And the syngas composition affects the optimal conversion rate of the chemical subsystem, the optimal point of which is around the stoichiometric composition for methanol production (CO/H = 0.5). In all, the polygeneration system fueled with coke oven gas and coal gas, which can realize the reasonable conversion of syngas to power and chemical product according to the syngas composition, is a promising method for coal energy conversion and utilization.

关键词： duo fuel of coke oven gas and coal gas     polygeneration of power and methanol     sensitivity analysis     the relation among energy utilization     syngas composition and chemical conversion rate    

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Effects of heavy rainfall on the composition of airborne bacterial communities

Gwang Il Jang, Chung Yeon Hwang, Byung Cheol Cho

《环境科学与工程前沿（英文）》 2018年 第12卷 第2期 doi: 10.1007/s11783-018-1008-0

摘要： Wet deposition scavenges particles and particle-associated bacteria from the air column, but the impact of raindrops on various surfaces on Earth causes emission of surface-associated bacteria into the air column. Thus, after rainfall, these two mechanisms are expected to cause changes in airborne bacterial community composition (BCC). In this study, aerosol samples were collected at a suburban site in Seoul, Korea before and after three heavy rainfall events in April, May, and July 2011. BCC was investigated by pyrosequencing the 16S rRNA gene in aerosol samples. Interestingly, the relative abundance of non-spore forming operational taxonomic units (OTUs) was always higher in post-rain aerosol samples. In particular, the absolute and relative abundances of airborne always increased after rainfall, whereas those of airborne , including and , consistently decreased. Marine bacterial sequences, which were temporally important in aerosol samples, also decreased after rainfall events. Further, increases in pathogen-like sequences were often observed in post-rain air samples. Rainfall events seemed to affect airborne BCCs by the combined action of the two mechanisms, with potentially adverse effects on human and plant health.

关键词： Aerosol     Bacteria     Community composition     Pyrosequencing     Rain    

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Syngas composition study

Zhe WANG , Jinning YANG , Zheng LI , Yong XIANG ,

《能源前沿（英文）》 2009年 第3卷 第3期   页码 369-372 doi: 10.1007/s11708-009-0044-7

摘要： The syngas composition characteristic was investigated in the real slurry-feed gasifier using a detailed gas phase reaction mechanism. The results show that the time for syngas to reach equilibrium is much shorter than the residence time for slurry feed entrained-flow gasifiers, indicating a gas phase species partial equilibrium state. Further calculation shows that the four major species, CO, CO, H, and HO, are in equilibrium via the reaction Bayu PRABOWO,Herri SUSANTO,Kentaro UMEKI,Mi YAN,Kunio YOSHIKAWA. [J]. Front. Energy, 2015, 9(3): 362-370.Ashok Jayawant Rao KECHE, Gaddale AMBA PRASAD RAO. [J]. Front Energ, 2013, 7(3): 300-306.Souman RUDRA, H. T. KIM, Jinwook LEE, L. ROSENDAHL, . [J]. Front. Energy, 2010, 4(3): 402-413. Fuchen WANG , Xinwen ZHOU , Wenyuan GUO , Zhenghua DAI , Xin GONG , Haifeng LIU , Zunhong YU , . [J]. Front. Energy, 2009, 3(1): 117-122.

关键词： entrained-flow     gasifier     syngas    

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Effect of wastewater composition on the calcium carbonate precipitation in upflow anaerobic sludge blanket

Shucheng YANG, Yanling HE, Charles CHOU, Pengxiang ZHANG, Dongqi WANG, Yonghong LIU,

《环境科学与工程前沿（英文）》 2010年 第4卷 第2期   页码 142-149 doi: 10.1007/s11783-010-0026-3

摘要： Calcium carbonate often precipitates in anaerobic reactors treating wastewater with high calcium content. The aim of this paper is to study the effect of wastewater composition on calcium carbonate precipitation in upflow anaerobic sludge blanket (UASB) reactors. Two laboratory-scale UASB reactors were operated with calcium-containing influents using acetate and carbohydrate as substrate, respectively. There was an obvious accumulation of inorganic precipitate observed in the biogranules. Observations via scanning electron microscope (SEM) and energy dispersive spectroscopy (EDS) showed that the acclimated biogranules in the two reactors differed in microstructure. Calcium carbonate was found to have precipitated on the surface of acetate-degrading biogranules, but precipitated at the core of the carbohydrate-degrading biogranules. The results indicated that substrates had significant influence on the location of calcium carbonate precipitation in anaerobic granular sludge, which was expected due to the different methanogens distribution and pH gradient within the granular sludge degrading various substrates. Moreover, the location of calcium carbonate precipitation substantially affected the specific methanogenic activity (SMA) of the granular sludge. The SMA of the acetate-degrading biogranules dropped from 1.96 gCOD·gVSS·d to 0.61 gCOD·gVSS·d after 180-d of operation in the reactor. However, the SMA of the carbohydrate-degrading biogranules was not adversely affected by calcium carbonate precipitation.

关键词： calcium carbonate     precipitation     anaerobic granular sludge     wastewater composition     microstructure     upflow anaerobic sludge blanket (UASB)    

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Development and applications of functional gene microarrays in the analysis of the functional diversity, composition

Zhili HE, Joy D. VAN NOSTRAND, Ye DENG, Jizhong ZHOU

《环境科学与工程前沿（英文）》 2011年 第5卷 第1期   页码 1-20 doi: 10.1007/s11783-011-0301-y

摘要： Functional gene arrays (FGAs) are a special type of microarrays containing probes for key genes involved in microbial functional processes, such as biogeochemical cycling of carbon, nitrogen, sulfur, phosphorus, and metals, biodegradation of environmental contaminants, energy processing, and stress responses. GeoChips are considered as the most comprehensive FGAs. Experimentally established probe design criteria and a computational pipeline integrating sequence retrieval, probe design and verification, array construction, data analysis, and automatic update are used to develop the GeoChip technology. GeoChip has been systematically evaluated and demonstrated to be a powerful tool for rapid, specific, sensitive, and quantitative analysis of microbial communities in a high-throughput manner. Several generations of GeoChip have been developed and applied to investigate the functional diversity, composition, structure, function, and dynamics of a variety of microbial communities from different habitats, such as water, soil, marine, bioreactor, human microbiome, and extreme ecosystems. GeoChip is able to address fundamental questions related to global change, bioenergy, bioremediation, agricultural operation, land use, human health, environmental restoration, and ecological theories and to link the microbial community structure to environmental factors and ecosystem functioning.

关键词： functional gene arrays (FGAs)     GeoChip     microbial communities     functional diversity/composition/structure     environmental factor     ecosystem functioning    

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Spent rechargeable lithium batteries in e-waste: composition and its implications

Xianlai ZENG,Jinhui LI

《环境科学与工程前沿（英文）》 2014年 第8卷 第5期   页码 792-796 doi: 10.1007/s11783-014-0705-6

摘要： The amount of spent rechargeable lithium batteries (RLBs) is growing rapidly owing to wide application of these batteries in portable electronic devices and electric vehicles, which obliges that spent RLBs should be handled properly. Identification of spent RLBs can supply fundamental information for spent RLBs recycling. This study aimed to determine the differences of physical components and chemical compositions among various spent RLBs. All the samplings of RLBs were rigorously dismantled and measured by an inductive coupled plasma atomic emission spectrometer. The results indicate that the average of total weight of the separator, the anode and the cathode accounted for over 60% of all the RLBs. The weight ratio of valuable metals ranged from 26% to 76%, and approximately 20% of total weight was Cu and Al. Moreover, no significant differences were found among different manufacturers, applications, and electrolyte types. And regarding portable electronic devices, there is also no significant difference in the Co-Li concentration ratios in the leaching liquid of RLBs.

关键词： rechargeable lithium batteries     e-waste     physical components     difference analysis     recycling    

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Visualization of amino acid composition differences between processed protein from different animal species

Xingfan ZHOU,Zengling YANG,Longjian CHEN,Lujia HAN

《农业科学与工程前沿（英文）》 2016年 第3卷 第2期   页码 171-179 doi: 10.15302/J-FASE-2016095

摘要： Amino acids are the dominant organic components of processed animal proteins, however there has been limited investigation of differences in their composition between various protein sources. Information on these differences will not only be helpful for their further utilization but also provide fundamental information for developing species-specific identification methods. In this study, self-organizing feature maps (SOFM) were used to visualize amino acid composition of fish meal, and meat and bone meal (MBM) produced from poultry, ruminants and swine. SOFM display the similarities and differences in amino acid composition between protein sources and effectively improve data transparency. Amino acid composition was shown to be useful for distinguishing fish meal from MBM due to their large concentration differences between glycine, lysine and proline. However, the amino acid composition of the three MBMs was quite similar. The SOFM results were consistent with those obtained by analysis of variance and principal component analysis but more straightforward. SOFM was shown to have a robust sample linkage capacity and to be able to act as a powerful means to link different sample for further data mining.

关键词： self-organizing feature maps     visualization     processed animal proteins (PAPs)     amino acid    

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Feasibility of crack free reinforced concrete bridge deck from materials composition perspective: a state

Mahdi AREZOUMANDI

《结构与土木工程前沿（英文）》 2015年 第9卷 第1期   页码 91-103 doi: 10.1007/s11709-015-0274-1

摘要： Early age cracking on bridge deck has been the subject of many studies for years. Cracking is a major concern because it leads to premature deterioration of structures. Millions of dollars spent to repair the cracked bridge decks each year. To design an appropriate mixture for crack free bridge deck, it is important to study previous researches. This paper presents a comprehensive literature review of the performance of different materials compositions as well as methods have been used to reduce and control bridge deck cracks. Different material compositions and methods are discussed in terms of their performances as well as advantages and disadvantages.

关键词： bridge deck     crack     fiber     shrinkage     shrinkage reducing admixture    

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湿地芦苇根系微生物群落组成与环境应用 Review

王东麟, 柏耀辉, 曲久辉

《工程（英文）》 2022年 第9卷 第2期   页码 42-50 doi: 10.1016/j.eng.2021.05.016

摘要：

芦苇是自然界广泛存在的湿地植物。在人工湿地中，约15.5%的种植植物是芦苇，其在废水水质净化中起到重要的作用。尽管如此，对芦苇根系微生物群落的基本组成及每一类微生物在污染物去除中的作用仍不清晰。本文总结了已有对芦苇根系微生物群落（包括细菌、古菌及真菌）在生态及生化方面的研究。基于下一代测序，对不同环境条件下的微生物群落组成进行了分析。此外，利用培养方法进一步研究了微生物群落的功能特征，如铁的固定、有机物的降解、营养元素的转化等。芦苇根系微生物群落独特的结构和功能受芦苇种类及盐度等环境因素的高度影响。基于现有对芦苇根系微生物群落的研究，我们建议在人工湿地中应用和强化合成微生物群落和铁锰氧化物基质，以提高湿地的水净化性能。

关键词： 芦苇     根系微生物     微生物群落组成     污染修复     人工湿地    

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标题 作者 时间 类型 操作

Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

期刊论文

Online single particle analysis of chemical composition and mixing state of crop straw burning particles

Juntao HUO,Xiaohui LU,Xinning WANG,Hong CHEN,Xingnan YE,Song Gao,Deborah S. Gross,Jianmin CHEN,Xin YANG

期刊论文

Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganese

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

期刊论文

Preliminary study of trace element emissions and control during coal combustion

ZHANG Junying, ZHAO Yongchun, DING Feng, ZENG Hancai, ZHENG Chuguang

期刊论文

“Composition” and regularisation of architectural production in contemporary China

Hua LI

期刊论文

Calorie restriction and its impact on gut microbial composition and global metabolism

Xiaojiao Zheng, Shouli Wang, Wei Jia

期刊论文

Sensitivity analysis of a methanol and power polygeneration system fueled with coke oven gas and coal gas

Guoqiang ZHANG, Lin GAO, Hongguang JIN, Rumou LIN, Sheng LI

期刊论文

Effects of heavy rainfall on the composition of airborne bacterial communities

Gwang Il Jang, Chung Yeon Hwang, Byung Cheol Cho

期刊论文

Syngas composition study

Zhe WANG , Jinning YANG , Zheng LI , Yong XIANG ,

期刊论文

Effect of wastewater composition on the calcium carbonate precipitation in upflow anaerobic sludge blanket

Shucheng YANG, Yanling HE, Charles CHOU, Pengxiang ZHANG, Dongqi WANG, Yonghong LIU,

期刊论文

Development and applications of functional gene microarrays in the analysis of the functional diversity, composition

Zhili HE, Joy D. VAN NOSTRAND, Ye DENG, Jizhong ZHOU

期刊论文

Spent rechargeable lithium batteries in e-waste: composition and its implications

Xianlai ZENG,Jinhui LI

期刊论文

Visualization of amino acid composition differences between processed protein from different animal species

Xingfan ZHOU,Zengling YANG,Longjian CHEN,Lujia HAN

期刊论文

Feasibility of crack free reinforced concrete bridge deck from materials composition perspective: a state

Mahdi AREZOUMANDI

期刊论文

湿地芦苇根系微生物群落组成与环境应用

王东麟, 柏耀辉, 曲久辉

期刊论文